RSC - Chem. Soc. Rev. latest articles

Supramolecular complexations of natural products

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60069F, Review Article

Hans-Jorg Schneider, Pawan Agrawal, Anatoly K. Yatsimirsky
Synthetic host compounds can efficiently complex natural products, such as a modified cyclodextrin with a bile acid or a cucurbituril with a peptide; they may be used e.g. for sensing, separation, enzyme assays, or drug protection. Also the host properties of some natural products find applications in analysis and separation.
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Thiol-addition reactions and their applications in thiol recognition

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60055F, Review Article

Caixia Yin, Fangjun Huo, Jingjing Zhang, Ramon Martinez-Manez, Yutao Yang, Haigang Lv, Sidian Li
Four reaction types, including 1,1, 1,2, 1,3, 1,4 addition reactions, based on different Michael acceptors have been used for the chromo-fluorogenic recognition of thiols.
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Recent progress in luminescent and colorimetric chemosensors for detection of thiols

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60024F, Tutorial Review

Hyo Sung Jung, Xiaoqiang Chen, Jong Seung Kim, Juyoung Yoon
This review focuses on the recent examples of fluorescent or colorimetric sensors for thiols, categorizing them based on diverse sensing mechanisms of optical probes towards thiols.
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Chemical information matters: an e-Research perspective on information and data sharing in the chemical sciences

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60050E, Review Article

Colin L. Bird, Jeremy G. Frey
A timely review of the information data sharing issue highlighted by the recent report about the research practices of chemists.
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Graphane and hydrogenated graphene

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60132C, Tutorial Review

Martin Pumera, Colin Hong An Wong
Do graphane and partially hydrogenated graphane possess the predicted properties? How to make graphane? What is graphane in the first place? Read here!
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Mechanochemistry of fullerenes and related materials

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS35494F, Review Article

San-E Zhu, Fei Li, Guan-Wu Wang
Functionalizations of fullerenes and related materials have been achieved by ball milling and hand grinding.
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Responsive hydrogels - structurally and dimensionally optimized smart frameworks for applications in catalysis, micro-system technology and material science

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60031A, Review Article

Artjom Doring, Wolfgang Birnbaum, Dirk Kuckling
The review covers the most recent developments in the field of responsive hydrogels focussing on catalysis, sensors and actuators.
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The modern interpretation of the Wittig reaction mechanism

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60105F, Review Article

Peter A. Byrne, Declan G. Gilheany
Li salt-free Wittig reactions of all ylide types occur under kinetic control, and by a common [2+2] cycloaddition mechanism in which oxaphosphetane is the first-formed and only intermediate.
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Mechanochemical organic synthesis

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS35526H, Review Article

Guan-Wu Wang
Various solvent-free mechanochemical organic reactions can be realized by ball milling techniques.
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Application of mass spectrometric techniques to delineate the modes-of-action of anticancer metallodrugs

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS35532B, Review Article

Christian G. Hartinger, Michael Groessl, Samuel M. Meier, Angela Casini, Paul J. Dyson
Mass spectrometric methods are increasingly being used to help elucidate the modes of action of metal-based anticancer agents. Nascent developments and recent applications are discussed in this review.
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Chemical routes to top-down nanofabrication

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60113G, Tutorial Review

Hai-Dong Yu, Michelle D. Regulacio, Enyi Ye, Ming-Yong Han
This tutorial review summarizes the different chemical routes to top-down nanofabrication that have enabled the construction of three-dimensional nanostructures with unique structural features and promising applications.
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Near-infrared phosphorescence: materials and applications

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60029G, Review Article

Haifeng Xiang, Jinghui Cheng, Xiaofeng Ma, Xiangge Zhou, Jason Joseph Chruma
An overview of the latest developments and applications in the field of room-temperature near-infrared phosphorescent transition-metal complexes is given.
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From powder to technical body: the undervalued science of catalyst scale up

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60076A, Review Article

Sharon Mitchell, Nina-Luisa Michels, Javier Perez-Ramirez
This review examines the complexity associated with the scale up of heterogeneous catalysts, proposing directions to strengthen the fundamental understanding of this exciting, but often neglected field.
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Multivalent scaffolds in glycoscience: an overview

Chem. Soc. Rev., 2013, 42,4515-4517
DOI: 10.1039/C3CS90029K, Editorial

Olivier Renaudet, Rene Roy
Guest editors Olivier Renaudet and Rene Roy introduce the Multivalent scaffolds in glycosciences themed issue of Chemical Society Reviews.
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How do multivalent glycodendrimers benefit from sulfur chemistry?

Chem. Soc. Rev., 2013, 42,4823-4841
DOI: 10.1039/C3CS60090D, Review Article

Marc Gingras, Yoann M. Chabre, Myriam Roy, Rene Roy
The combination of sugar and sulfur chemistry is reported to benefit multivalent glycodendrimer chemistry. Besides the contribution of sulfur to structural linking strategies, we emphasized some novelties in the modulation of optoelectronic properties of those ligands and their uses in glycobiology, in materials science and in nanoscience.
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Multivalent glycoliposomes and micelles to study carbohydrate-protein and carbohydrate-carbohydrate interactions

Chem. Soc. Rev., 2013, 42,4640-4656
DOI: 10.1039/C3CS00001J, Tutorial Review

Narayanaswamy Jayaraman, Krishnagopal Maiti, Kottari Naresh
The synthetic design of glycolipids, and formation of glycoliposomes and micelles thereof to study multivalent carbohydrate-protein and carbohydrate-carbohydrate interactions are presented.
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Multivalent glycoconjugate syntheses and applications using aromatic scaffolds

Chem. Soc. Rev., 2013, 42,4657-4708
DOI: 10.1039/C3CS35483K, Review Article

Yoann M. Chabre, Rene Roy
This review describes the chemical syntheses and biological properties of multivalent glycoarchitectures prepared around aromatic backbones.
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Glycopeptide dendrimers as Pseudomonas aeruginosa biofilm inhibitors

Chem. Soc. Rev., 2013, 42,4814-4822
DOI: 10.1039/C3CS35504G, Review Article

Jean-Louis Reymond, Myriam Bergmann, Tamis Darbre
Inhibition and dispersal of Pseudomonas aeruginosa biofilms were achieved with multivalent glycopeptide dendrimer inhibitors of lectins LecA and LecB.
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Multivalent glycocalixarenes for recognition of biological macromolecules: glycocalyx mimics capable of multitasking

Chem. Soc. Rev., 2013, 42,4623-4639
DOI: 10.1039/C2CS35437C, Tutorial Review

Francesco Sansone, Alessandro Casnati
Glycocalixarenes, like the cell-wall glycocalyx, recognise macromolecules through multivalency. Their possibility to simultaneously perform other tasks such as drug-delivery, imaging or immunostimulation suggests their potential application in bionanotechnology and nanomedicine.
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Binding sugars: from natural lectins to synthetic receptors and engineered neolectins

Chem. Soc. Rev., 2013, 42,4798-4813
DOI: 10.1039/C2CS35435G, Review Article

Julie Arnaud, Aymeric Audfray, Anne Imberty
From structural knowledge of natural lectins, artificial carbohydrate-binders are developed based either on engineered biomolecules or on biomimetics systems.
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Enzymatic glycosylation of multivalent scaffolds

Chem. Soc. Rev., 2013, 42,4774-4797
DOI: 10.1039/C2CS35395D, Review Article

Pavla Bojarova, Ruben R. Rosencrantz, Lothar Elling, Vladimir Kren
The use of glycosyltransferases for glycosylating natural and synthetic multivalent substrates is presented, including glycoarrays, metabolic labeling and glycosylation engineering.
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Cyclodextrin-based multivalent glycodisplays: covalent and supramolecular conjugates to assess carbohydrate-protein interactions

Chem. Soc. Rev., 2013, 42,4746-4773
DOI: 10.1039/C2CS35424A, Review Article

Alvaro Martinez, Carmen Ortiz Mellet, Jose M. Garcia Fernandez
Multivalent cyclodextrin conjugates, from covalent to self-assembled constructs, can be tailored to investigate and control carbohydrate binding to biological receptors.
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Glyconanoparticles as multifunctional and multimodal carbohydrate systems

Chem. Soc. Rev., 2013, 42,4728-4745
DOI: 10.1039/C2CS35420A, Review Article

Marco Marradi, Fabrizio Chiodo, Isabel Garcia, Soledad Penades
Glyconanoparticles with varying density of carbohydrates are multivalent and multifunctional tools for studying interactions, for developing vaccines, and for molecular imaging.
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Bacterial toxin inhibitors based on multivalent scaffolds

Chem. Soc. Rev., 2013, 42,4613-4622
DOI: 10.1039/C2CS35430F, Tutorial Review

Thomas R. Branson, W. Bruce Turnbull
Protein toxins released by certain intestinal bacteria are the cause of many diarrhoeal diseases including cholera and travellers' diarrhoea.
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Multivalent glyco(cyclo)peptides

Chem. Soc. Rev., 2013, 42,4599-4612
DOI: 10.1039/C2CS35413F, Tutorial Review

M. Carmen Galan, Pascal Dumy, Olivier Renaudet
This tutorial review provides an overview of the most recent advances in the preparation and utilization of glycopeptides and glycocyclopeptides in glycobiology.
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Carbosilane glycodendrimers

Chem. Soc. Rev., 2013, 42,4574-4598
DOI: 10.1039/C2CS35421G, Tutorial Review

Ken Hatano, Koji Matsuoka, Daiyo Terunuma
Glycodendrimers fascinate both carbohydrate chemists and biologists because of their ability to recognize lectins and enhance carbohydrate-protein interactions.
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Glycoclusters on oligonucleotide and PNA scaffolds: synthesis and applications

Chem. Soc. Rev., 2013, 42,4557-4573
DOI: 10.1039/C2CS35406C, Tutorial Review

Nicolas Spinelli, Eric Defrancq, Francois Morvan
Oligonucleotide glycocluster conjugates are involved in several approaches for cellular delivery, carbohydrate microarray or supramolecular glycoclusters.
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Multivalent glycoconjugates as anti-pathogenic agents

Chem. Soc. Rev., 2013, 42,4709-4727
DOI: 10.1039/C2CS35408J, Review Article

Anna Bernardi, Jesus Jimenez-Barbero, Alessandro Casnati, Cristina De Castro, Tamis Darbre, Franck Fieschi, Jukka Finne, Horst Funken, Karl-Erich Jaeger, Martina Lahmann, Thisbe K. Lindhorst, Marco Marradi, Paul Messner, Antonio Molinaro, Paul V. Murphy, Cristina Nativi, Stefan Oscarson, Soledad Penades, Francesco Peri, Roland J. Pieters, Olivier Renaudet, Jean-Louis Reymond, Barbara Richichi, Javier Rojo, Francesco Sansone, Christina Schaffer, W. Bruce Turnbull, Trinidad Velasco-Torrijos, Sebastien Vidal, Stephane Vincent, Tom Wennekes, Han Zuilhof, Anne Imberty
Glycocompounds interfere with infection and immunity.
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Clustered carbohydrates in synthetic vaccines

Chem. Soc. Rev., 2013, 42,4543-4556
DOI: 10.1039/C2CS35422E, Tutorial Review

Francesco Peri
Are there general rules for the design of efficient carbohydrate vaccines? Recent achievements in the field of carbohydrate immunization.
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Sweet carbon nanostructures: carbohydrate conjugates with carbon nanotubes and graphene and their applications

Chem. Soc. Rev., 2013, 42,4532-4542
DOI: 10.1039/C2CS35396B, Tutorial Review

Yanan Chen, Alexander Star, Sebastien Vidal
This review highlights the strategies for the covalent and noncovalent functionalization of carbon nanostructures with carbohydrates and applications in biology.
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Multivalency in heterogeneous glycoenvironments: hetero-glycoclusters, -glycopolymers and -glycoassemblies

Chem. Soc. Rev., 2013, 42,4518-4531
DOI: 10.1039/C2CS35219B, Tutorial Review

Jose L. Jimenez Blanco, Carmen Ortiz Mellet, Jose M. Garcia Fernandez
"Shuffled", multidomain and fluidic displays of different glycotopes allow assessing the effect of heterogeneity in carbohydrate-lectin or -antibody interactions.
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Alkaline polymer electrolyte membranes for fuel cell applications

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60053J, Review Article

Yan-Jie Wang, Jinli Qiao, Ryan Baker, Jiujun Zhang
In this review, we examine the most recent progress in the area of alkaline polymer electrolyte membrane (PEM) development in terms of material selection, synthesis, characterization, and theoretical approach, as well as their fabrication into alkaline PEM-based membrane electrode assemblies and the corresponding fuel cell performance.
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Magnetic responsive polymer composite materials

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60058K, Tutorial Review

Julie Thevenot, Hugo Oliveira, Olivier Sandre, Sebastien Lecommandoux
Magnetic responsive materials and their potential breakthrough applications in the biomedical, coatings, microfluidics and microelectronics fields are highlighted in this review.
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Stimuli responsive synthetic polypeptides derived from N-carboxyanhydride (NCA) polymerisation

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60063G, Review Article

Jin Huang, Andreas Heise
Advanced polymerisation and modification approaches have opened new avenues to produce novel biologically inspired responsive synthetic polypeptides.
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Proteotyping for the rapid identification of influenza virus and other biopathogens

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60081E, Tutorial Review

Kevin M. Downard
A new proteotyping approach to characterise the influenza virus, and by extension other biopathogens, through the detection of signature peptides.
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Ubiquitous trisulfur radical anion: fundamentals and applications in materials science, electrochemistry, analytical chemistry and geochemistry

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60119F, Tutorial Review

Tristram Chivers, Philip J. W. Elder
The fundamental chemistry and multi-faceted influence of the paramagnetic, deep blue sulfur species [S₃][radical dot]^- in materials science, electrochemistry, analytical chemistry and geochemistry are discussed.
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Dendritic architectures based on bis-MPA: functional polymeric scaffolds for application-driven research

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60101C, Review Article

Anna Carlmark, Eva Malmstrom, Michael Malkoch
This review covers the array of synthetic methodologies as well as potential applications of dendritic architectures based on bis-MPA.
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An overview of the magnetoresistance phenomenon in molecular systems

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60074B, Review Article

Hongbo Gu, Xi Zhang, Huige Wei, Yudong Huang, Suying Wei, Zhanhu Guo
Magnetoresistance effects in molecular systems are summarized and the related models are reviewed together with some detailed application examples.
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Heteroarenes as high performance organic semiconductors

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60108K, Review Article

Wei Jiang, Yan Li, Zhaohui Wang
This review article highlights the practical synthesis, tuneable self-assembled packing arrangement and high electronic performance of heteroarenes.
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Carbohydrate chemistry

Chem. Soc. Rev., 2013, 42,4267-4269
DOI: 10.1039/C3CS90030D, Editorial

Injae Shin, Kwan Soo Kim
Guest editors Injae Shin and Kwan Soo Kim introduce the Carbohydrate chemistry themed issue of Chemical Society Reviews.
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Bridging lectin binding sites by multivalent carbohydrates

Chem. Soc. Rev., 2013, 42,4492-4503
DOI: 10.1039/C3CS60089K, Review Article

Valentin Wittmann, Roland J. Pieters
Creating potent bridging ligands for medicinally important lectins is a strategy that increasingly sees creative and successful examples that are highlighted here.
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Glycopolymer probes of signal transduction

Chem. Soc. Rev., 2013, 42,4476-4491
DOI: 10.1039/C3CS60097A, Review Article

Laura L. Kiessling, Joseph C. Grim
This review begins with an overview of the structural features of glycopolymers that can affect their recognition by protein receptors and then highlights the use of glycopolymers as probes of signal transduction.
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Development of fucosyltransferase and fucosidase inhibitors

Chem. Soc. Rev., 2013, 42,4459-4475
DOI: 10.1039/C3CS60056D, Review Article

Zhijay Tu, Yu-Nong Lin, Chun-Hung Lin
We provide an updated review of the development of fucosyltransferase and fucosidase inhibitors with an emphasis on the structure-activity relationship.
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Lectin microarrays: concept, principle and applications

Chem. Soc. Rev., 2013, 42,4443-4458
DOI: 10.1039/C3CS35419A, Review Article

Jun Hirabayashi, Masao Yamada, Atsushi Kuno, Hiroaki Tateno
The lectin microarray is a novel technology that enables rapid and high-sensitivity profiling of complex features of glycans without their liberation.
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The development of synthetic antitumour vaccines from mucin glycopeptide antigens

Chem. Soc. Rev., 2013, 42,4421-4442
DOI: 10.1039/C3CS35470A, Review Article

Nikola Gaidzik, Ulrika Westerlind, Horst Kunz
Synthetic vaccines containing glycopeptide antigens from tumour-associated mucins and immunostimulatory components induce strong immune responses directed towards tumour cells.
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Chemical assembly of N-glycoproteins: a refined toolbox to address a ubiquitous posttranslational modification

Chem. Soc. Rev., 2013, 42,4408-4420
DOI: 10.1039/C3CS35485G, Review Article

Carlo Unverzagt, Yasuhiro Kajihara
Recent developments in the ligation chemistry of peptides and carbohydrates have enabled researchers to assemble entire glycoproteins with high precision.
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Design of chemical glycosyl donors: does changing ring conformation influence selectivity/reactivity?

Chem. Soc. Rev., 2013, 42,4297-4309
DOI: 10.1039/C3CS35457A, Tutorial Review

Hiroko Satoh, Shino Manabe
This tutorial review focuses on the design of glycosyl donors, especially on attempts to control selectivity/reactivity by employing bulky substituents, cyclic protecting groups, or bridged structures.
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The biosynthesis of nitrogen-, sulfur-, and high-carbon chain-containing sugars

Chem. Soc. Rev., 2013, 42,4377-4407
DOI: 10.1039/C2CS35438A, Review Article

Chia-I. Lin, Reid M. McCarty, Hung-wen Liu
This review provides an update of current understanding of the biosynthesis of nitrogen-, sulfur-, high-carbon chain-containing sugars.
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Glyconanotechnology

Chem. Soc. Rev., 2013, 42,4358-4376
DOI: 10.1039/C2CS35427F, Review Article

Niels C. Reichardt, Manuel Martin-Lomas, Soledad Penades
The most recent developments of glyconanomaterials for drug design, vaccine development, molecular imaging, enzyme inhibition and biosensors are critically discussed.
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Chemical probing of glycans in cells and organisms

Chem. Soc. Rev., 2013, 42,4284-4296
DOI: 10.1039/C2CS35416K, Tutorial Review

Sara H. Rouhanifard, Lars Ulrik Nordstrom, Tianqing Zheng, Peng Wu
New chemical tools have made it possible to probe glycans in living systems.
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Chemical approaches to study O-GlcNAcylation

Chem. Soc. Rev., 2013, 42,4345-4357
DOI: 10.1039/C2CS35412H, Review Article

Partha S. Banerjee, Gerald W. Hart, Jin Won Cho
The chemistry of O-GlcNAc, the cycling enzymes and some of the methods developed to study protein O-GlcNAc modifications are described.
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Designing a new antifungal glycoconjugate vaccine

Chem. Soc. Rev., 2013, 42,4327-4344
DOI: 10.1039/C2CS35382B, Review Article

Margaret A. Johnson, David R. Bundle
New strategies for binding site mapping and for eliciting protective immune responses against small carbohydrate epitopes are reviewed.
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Fluoro-C-glycosides and fluoro-carbasugars, hydrolytically stable and synthetically challenging glycomimetics

Chem. Soc. Rev., 2013, 42,4270-4283
DOI: 10.1039/C2CS35403A, Tutorial Review

Eric Leclerc, Xavier Pannecoucke, Melanie Etheve-Quelquejeu, Matthieu Sollogoub
Fluoro-C-glycosides and fluoro-carbasugars are a particular subclass of hydrolytically stable glycomimetics that are expected to have different, hopefully improved properties thanks to the stereoelectronic features of the fluoroalkyl moiety.
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Carbohydrate microarrays

Chem. Soc. Rev., 2013, 42,4310-4326
DOI: 10.1039/C2CS35401B, Review Article

Sungjin Park, Jeffrey C. Gildersleeve, Ola Blixt, Injae Shin
This article discusses construction of carbohydrate microarrays, detection methods of carbohydrate microarrays and their applications in biological and biomedical research.
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Microfluidics and Raman microscopy: current applications and future challenges

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS35515B, Review Article

Adam F. Chrimes, Khashayar Khoshmanesh, Paul R. Stoddart, Arnan Mitchell, Kourosh Kalantar-zadeh
This critical review discusses the integration of Raman microscopy with microfluidics - its methods and applications.
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Adaptive all the way down: Building responsive materials from hierarchies of chemomechanical feedback

Chem. Soc. Rev., 2013, Advance Article
DOI: 10.1039/C3CS60045A, Tutorial Review

Alison Grinthal, Joanna Aizenberg
We explore how feedback between chemistry and motion can be harnessed to design an unlimited diversity of multi-responsive, multifunctional systems with adaptiveness built in from the bottom up.
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